Freezing and Scraping the Stain
Put the clothing in the freezer. If you don't notice the stain for several days, place the garment in the freezer for a few hours. This will cause the caulk to harden. After a few days, you should be able to easily "peel" most of the goop off with your fingernails or a butter knife. Once the caulk is solid, carefully peel it off the article of clothing. The biggest chunk should come off in a glob. Alternately, use an ice cube. Hold an ice cube in place over the stain until it freezes. Once frozen, the caulk will loosen and can be pulled off more easily.
Scrape the stain from the clothing with scissors. Chip away at the caulk, bit by bit – this may be easier once the stain is frozen. You can also use a butter knife, a file, or another scraping tool. Be careful not to cut yourself or the clothing! If you're wearing cotton and caulk gets on the outside surface of your clothes, you can usually just peel it off. If you're wearing cotton and the caulk gets into the fibers of your clothes, it'll be difficult to remove but you can probably brush it.
Finish the job. After the excess is removed, clean any remaining stain with rubbing alcohol or another cleaning agent. You should be able to scrape or peel off the bulk, but some stain might remain.
Blotting the Stain
Tackle the caulk stain as quickly as possible. If you notice the stains before it has a chance to dry, you might be more likely to remove it all. Try running your clothing through a regular washing cycle in your washing machine with standard detergent. If the clothing is white, add bleach for extra washing power. New caulk stains or ones that have not completely dried may come off with a normal wash.
Blot the stain with water. Wet a rag or a paper towel. Press the towel firmly against the caulk, and let the moisture sink in. Dab the area again and again, and gently rub the stain out of the fabric. Try to blot as much of the caulk as possible off of the garment.
Dab the caulk with rubbing alcohol. After you have removed as much excess caulk as you can, wet a piece of folded paper towel with some rubbing alcohol. Blot the stain, firmly, and let the alcohol soak deep into the fabric. Dab the stain as many times as needed to remove the stain. You may need to reapply several times to remove the stain. Add more alcohol each time. Always use a clean section of the towel. If the towel becomes overly stained and saturated with caulk, you may need to switch to another rag.
Wash the clothing. Once the stain is removed, launder the garment in cold or warm water. When you remove the garment from the washer, examine the stain to make sure it's completely removed. You may have to wash it a few times to get the stain completely out. Don't place it in a dryer with any stain remaining, since the heat will set it.
Other Methods
Use a chemical cleaner. Purchase a commercial cleaner, such as Goof Off Stain Remover, to finish the job. Look for specific caulk removers. Follow all instructions and warnings supplied by the manufacturer to ensure proper cleaning. Warning: Always pretest new cleaners on old clothing before applying it to important or favorite garments.
Try using hand sanitizer. Antibacterial sanitizing products can remove some stains from clothing, and they may be effective on caulk. First, squeeze the sanitizer onto the stained area. Rub the spot gently with a tissue or a damp rag. You may need to use several applications of sanitizer if the stain is especially bad.
Rub with baking soda. Wet the stain with water. Pour baking soda onto the fabric while it's still wet. Massage the baking soda into the fabric with a rag or towel until the caulk comes out. If the stain does not come out completely, keep trying. Put the clothing in the wash afterward, and results will improve even more.
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